Dimethyl sulfide in the Amazon rain forest

Jardine, Kolby J.; Yáñez-Serrano, Ana Maria; Williams, Jonathan C.; Kunert, Norbert; Jardine, Angela B.; Taylor, Tyeen C.; Abrell, Leif; Artaxo, Paulo; Guenther, Alex B.; Hewitt, Nick; House, Emily R.; Florentino, A. P.; Manzi, Antônio Ocimar; Higuchi, Niro; Kesselmeier, Jürgen; Behrendt, Thomas; Veres, Patrick R.; Derstroff, Bettina; Fuentes, José D.; Martin, Scot T.; Andreae, Meinrat O.

Artigo

Dimethyl sulfide in the Amazon rain forest

Surface-to-atmosphere emissions of dimethyl sulfide (DMS) may impact global climate through the formation of gaseous sulfuric acid, which can yield secondary sulfate aerosols and contribute to new particle formation. While oceans are generally considered the dominant sources of DMS, a shortage of ec...

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Autor principal:	Jardine, Kolby J.
Outros Autores:	Yáñez-Serrano, Ana Maria, Williams, Jonathan C., Kunert, Norbert, Jardine, Angela B., Taylor, Tyeen C., Abrell, Leif, Artaxo, Paulo, Guenther, Alex B., Hewitt, Nick, House, Emily R., Florentino, A. P., Manzi, Antônio Ocimar, Higuchi, Niro, Kesselmeier, Jürgen, Behrendt, Thomas, Veres, Patrick R., Derstroff, Bettina, Fuentes, José D., Martin, Scot T., Andreae, Meinrat O.
Grau:	Artigo
Idioma:	English
Publicado em:	Global Biogeochemical Cycles 2020
Assuntos:	Air-soil Interaction Biogenic Emission Biogeochemistry Climate Feedback Dimethylsulfide Mixing Ratio Rainforest Soil Emission Spatio-temporal Analysis Sulfuric Acid Amazon Basin
Acesso em linha:	https://repositorio.inpa.gov.br/handle/1/15969

id	oai:repositorio:1-15969
recordtype	dspace
spelling	oai:repositorio:1-15969 Dimethyl sulfide in the Amazon rain forest Jardine, Kolby J. Yáñez-Serrano, Ana Maria Williams, Jonathan C. Kunert, Norbert Jardine, Angela B. Taylor, Tyeen C. Abrell, Leif Artaxo, Paulo Guenther, Alex B. Hewitt, Nick House, Emily R. Florentino, A. P. Manzi, Antônio Ocimar Higuchi, Niro Kesselmeier, Jürgen Behrendt, Thomas Veres, Patrick R. Derstroff, Bettina Fuentes, José D. Martin, Scot T. Andreae, Meinrat O. Air-soil Interaction Biogenic Emission Biogeochemistry Climate Feedback Dimethylsulfide Mixing Ratio Rainforest Soil Emission Spatio-temporal Analysis Sulfuric Acid Amazon Basin Surface-to-atmosphere emissions of dimethyl sulfide (DMS) may impact global climate through the formation of gaseous sulfuric acid, which can yield secondary sulfate aerosols and contribute to new particle formation. While oceans are generally considered the dominant sources of DMS, a shortage of ecosystem observations prevents an accurate analysis of terrestrial DMS sources. Using mass spectrometry, we quantified ambient DMS mixing ratios within and above a primary rainforest ecosystem in the central Amazon Basin in real-time (2010-2011) and at high vertical resolution (2013-2014). Elevated but highly variable DMS mixing ratios were observed within the canopy, showing clear evidence of a net ecosystem source to the atmosphere during both day and night in both the dry and wet seasons. Periods of high DMS mixing ratios lasting up to 8 h (up to 160 parts per trillion (ppt)) often occurred within the canopy and near the surface during many evenings and nights. Daytime gradients showed mixing ratios (up to 80 ppt) peaking near the top of the canopy as well as near the ground following a rain event. The spatial and temporal distribution of DMS suggests that ambient levels and their potential climatic impacts are dominated by local soil and plant emissions. A soil source was confirmed by measurements of DMS emission fluxes from Amazon soils as a function of temperature and soil moisture. Furthermore, light- and temperature-dependent DMS emissions were measured from seven tropical tree species. Our study has important implications for understanding terrestrial DMS sources and their role in coupled land-atmosphere climate feedbacks. © 2014. The Authors. 2020-05-21T20:06:17Z 2020-05-21T20:06:17Z 2015 Artigo https://repositorio.inpa.gov.br/handle/1/15969 10.1002/2014GB004969 en Volume 29, Número 1, Pags. 19-32 Attribution-NonCommercial-NoDerivs 3.0 Brazil http://creativecommons.org/licenses/by-nc-nd/3.0/br/ application/pdf Global Biogeochemical Cycles
institution	Instituto Nacional de Pesquisas da Amazônia - Repositório Institucional
collection	INPA-RI
language	English
topic	Air-soil Interaction Biogenic Emission Biogeochemistry Climate Feedback Dimethylsulfide Mixing Ratio Rainforest Soil Emission Spatio-temporal Analysis Sulfuric Acid Amazon Basin
spellingShingle	Air-soil Interaction Biogenic Emission Biogeochemistry Climate Feedback Dimethylsulfide Mixing Ratio Rainforest Soil Emission Spatio-temporal Analysis Sulfuric Acid Amazon Basin Jardine, Kolby J. Dimethyl sulfide in the Amazon rain forest
topic_facet	Air-soil Interaction Biogenic Emission Biogeochemistry Climate Feedback Dimethylsulfide Mixing Ratio Rainforest Soil Emission Spatio-temporal Analysis Sulfuric Acid Amazon Basin
description	Surface-to-atmosphere emissions of dimethyl sulfide (DMS) may impact global climate through the formation of gaseous sulfuric acid, which can yield secondary sulfate aerosols and contribute to new particle formation. While oceans are generally considered the dominant sources of DMS, a shortage of ecosystem observations prevents an accurate analysis of terrestrial DMS sources. Using mass spectrometry, we quantified ambient DMS mixing ratios within and above a primary rainforest ecosystem in the central Amazon Basin in real-time (2010-2011) and at high vertical resolution (2013-2014). Elevated but highly variable DMS mixing ratios were observed within the canopy, showing clear evidence of a net ecosystem source to the atmosphere during both day and night in both the dry and wet seasons. Periods of high DMS mixing ratios lasting up to 8 h (up to 160 parts per trillion (ppt)) often occurred within the canopy and near the surface during many evenings and nights. Daytime gradients showed mixing ratios (up to 80 ppt) peaking near the top of the canopy as well as near the ground following a rain event. The spatial and temporal distribution of DMS suggests that ambient levels and their potential climatic impacts are dominated by local soil and plant emissions. A soil source was confirmed by measurements of DMS emission fluxes from Amazon soils as a function of temperature and soil moisture. Furthermore, light- and temperature-dependent DMS emissions were measured from seven tropical tree species. Our study has important implications for understanding terrestrial DMS sources and their role in coupled land-atmosphere climate feedbacks. © 2014. The Authors.
format	Artigo
author	Jardine, Kolby J.
author2	Yáñez-Serrano, Ana Maria Williams, Jonathan C. Kunert, Norbert Jardine, Angela B. Taylor, Tyeen C. Abrell, Leif Artaxo, Paulo Guenther, Alex B. Hewitt, Nick House, Emily R. Florentino, A. P. Manzi, Antônio Ocimar Higuchi, Niro Kesselmeier, Jürgen Behrendt, Thomas Veres, Patrick R. Derstroff, Bettina Fuentes, José D. Martin, Scot T. Andreae, Meinrat O.
author2Str	Yáñez-Serrano, Ana Maria Williams, Jonathan C. Kunert, Norbert Jardine, Angela B. Taylor, Tyeen C. Abrell, Leif Artaxo, Paulo Guenther, Alex B. Hewitt, Nick House, Emily R. Florentino, A. P. Manzi, Antônio Ocimar Higuchi, Niro Kesselmeier, Jürgen Behrendt, Thomas Veres, Patrick R. Derstroff, Bettina Fuentes, José D. Martin, Scot T. Andreae, Meinrat O.
title	Dimethyl sulfide in the Amazon rain forest
title_short	Dimethyl sulfide in the Amazon rain forest
title_full	Dimethyl sulfide in the Amazon rain forest
title_fullStr	Dimethyl sulfide in the Amazon rain forest
title_full_unstemmed	Dimethyl sulfide in the Amazon rain forest
title_sort	dimethyl sulfide in the amazon rain forest
publisher	Global Biogeochemical Cycles
publishDate	2020
url	https://repositorio.inpa.gov.br/handle/1/15969
_version_	1787144888772460544
score	11.671464

Dimethyl sulfide in the Amazon rain forest

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